The purpose of this post is to provide estimates of the plutonium (Pu) isotopes present at the Fukushima Dai-ichi nuclear power plant (NPP) at the beginning of the disaster in March 2011. The post is part of an ongoing effort to communicate facts about Fukushima obtained through scientific study of the impact of the meltdowns on the environment. Comments on this site and in other public forums highlight the fact that Unit 3 at the NPP was burning mixed oxide (MOX) fuel at the time of the accident which, because it is enriched in Pu, suggests that these releases are potentially more harmful. Here I report estimates of Pu present in the reactors (Units 1, 2 and 3) and spent fuel pools (Units 1-4) at the site based on burnup calculations. Because fission of low enriched uranium (LEU) fuel produces Pu isotopes during operation there was a significant amount of Pu on site in Units 1-4. During extended operation a MOX fuel burning reactor can produce multiple times the Pu of LEU but this was not so at the time of the Fukushima meltdowns. The amount of additional Pu present due to Unit 3’s MOX fuel is small compared to the other reactor cores and the inventory of the spent fuel pools. The differences between environmental impact of MOX versus LEU reactor core meltdown in this case are small. Estimates of the release of Pu isotopes from Fukushima, based on measurements of air, soil and water suggest 100,000 fold less was broadcast to the environment compared to Chernobyl and 5,000,000 fold lower than releases from nuclear weapons testing in the 20th century. Continue reading Plutonium Inventories at Fukushima Dai-ichi Nuclear Power Plant and Mixed Oxide (MOX) Fuel at Unit 3
The purpose of this diary is to summarize recent models and measurements of the release of strontium-90 (90-Sr, half life 28.8 yr) to the ocean resulting from the triple meltdowns at the Fukushima-Daiichi nuclear power plant in March 2011. This post is part of an ongoing series aimed at understanding the impact of the disaster on the North Pacific Ocean and residents of the west coast of North America. 90-Sr is a beta-emitting element that is a radiological health concern given its relatively long half life and similar chemistry to the nutrient calcium (Ca). Previous peer-reviewed work indicate that releases of 90-Sr were about 30-10,000 fold less than 137-Cs and similar to the release of 90-Sr from the Chernobyl disaster in 1986 and about 600-fold lower than the releases from atmospheric weapons tests that peaked in the mid-1960’s. Given maximal release rates after the disaster, modeled activities of 90-Sr in the marine foodweb and in fish that accounts for bioconcentration and accumulation predict maximal dose rates from Fukushima to human consumers three orders of magnitude less than doses owing to the presence of 137-Cs in marine products and thus well below maximum dose limits thought to be detrimental to public health. Continue reading Release, Dispersion and Fate of Radioactive Strontium From Fukushima in the Northwest Pacific Ocean
One of the goals of the InFORM project is to make measurements of radionuclides in the North Pacific Ocean to determine maximum activities that will determine impacts on the marine ecosystem and residents of the west coast. The purpose of this post is to bring to the attention of readers a recently published correction to a prominent model that predicts the activity of Fukushima derived Cesium-137 (137-Cs, half life ~30 years) in seawater of the North Pacific. The diary is part of an ongoing series aimed at discussing research addressing the impact of the Fukushima nuclear disaster on the health of the North Pacific Ocean and inhabitants of North America’s west coast. Predictions of a model by Rossi and colleagues published in Deep-Sea Research in 2013 of the evolution of the plume of seawater contaminated by the Fukushima triple meltdowns are an order of magnitude too high. Rather than a range of ~1-30 Bq/m^3 reported previously maximum activities off the west coast of North America are likely to be ~3 Bq/m^3 or about more than 25 times lower than maximum activities measured in the Pacific in the mid-20th century resulting from atmospheric weapons tests. These activities are not likely to represent significant radiological health risks to the North Pacific ecosystem or residents of the North American west coast.
A paper by Rossi et al. (2013) used a Lagrangian model to predict the temporal and spatial evolution of the seawater plume contaminated by the Fukushima nuclear disaster beginning in March 2011. The model predicted a range of 10-30 Bq/m^3 137-Cs in waters off the coast of North America at 49 degrees North latitude as demonstrated in the figure shown below:
This model predicted higher maximum 137-Cs activities in seawater in the North Pacific compared with a similar model published by Behrens et al. (2012) that had maximum activities off of North America reaching only ~1-2 Bq/m^3.
Recently, after comments from Professor Michio Aoyama of Japan, Rossi and colleagues recognized an error in their model and have published a correction to their 2013 study here. The error resulted in a factor of 10 overestimation of maximum activities of 137-Cs in the Pacific such that maximum 137-Cs off N. America will likely be between 1 and 3 Bq/m^3. The corrections to the model do not affect the conclusions of the study and results from the 2013 study are easy scaled to the more accurate values given the Langrangian approach used by the authors in the original work.
The figure below shows the time evolution of the plume at various latitudes along the international date line and compares the model output with measurements made by Aoyama et al. (2013) along the international dateline at about 40 degrees N in 2012.
The factor of 10 lower activity correction better agrees with the Behrens et al. (2012) modeling study and measurements of 137-Cs in seawater made by Japanese and North American scientists.
Maximum activities of ~1-3 Bq/m^3 as the heart of the contaminated plume reaches the North American coast in the coming 2 year period are roughly 25-fold lower than 137-Cs activities in the North Pacific circa 1960 resulting from atmospheric weapons testing. Therefore, it is unlikely that 137-Cs activities of 3 Bq/m^3 or associated radionuclides released at lower total activities from Fukushima will represent significant health risks to the North Pacific ecosystem.
Ongoing monitoring of radionuclide activities in the North Pacific is required to ground-truth models of Pacific Ocean circulation and plume evolution and to provide the best information to determine likely impact to residents of North America.
This post is part of an ongoing series that endeavors to provide useful and accurate information about: 1) the fate of Fukushima derived radionuclides in the Pacific Ocean, and, 2) the impact of these radionuclides on the marine ecosystem and the west coast of North America. The purpose of this diary is to draw attention to a number of poorly researched posts about a recently published study (unfortunately this study is behind a publisher pay-wall) in a Chinese journal that predicts a concentrated plume of radioactive elements from Fukushima arriving on the west coast. It is an unfortunate but common example of how news aggregation sites can misinterpret the results of a scientific study and misinform the public.
What models can and cannot say about the Fukushima plume
The study in question by Fu and co-workers published in the Journal of Ocean University of China in 2014 (behind pay-wall unfortunately) is wholly incapable of describing the behavior of dissolved radionuclides in the plume that is now arriving on the west coast of North America.
From the paper the authors themselves state in the methods that:
“In the study, the radioactive pollutant in the ocean is treated as a mixture of multiple Lagrangian particulates, and each particulate represents a radioactive element. The particulates can move in both horizontal and vertical directions, but cannot diffuse and mix with surrounding seawater.”
What this means is that rather than being allowed to mix and diffuse (or decay or sink after becoming associated with particles) the radionuclides are treated as neutrally buoyant drifters. The model, therefore, greatly overestimates the concentrations of radionuclides reaching the west coast of North America in the plume.
For those interested in models using accurate physics that will allow for an accurate prediction of radionuclide concentrations consult the following studies:
The Behrens et al. study is open-access while the Rossi et al. study is not. Measurements taken in the North Pacific by Canada’s Department of Fisheries and Oceans and InFORM team member Dr. John Smith indicate that the Rossi et al. study predicts the arrival time of the plume on the west coast but overestimates the activity of the Fukushima derived radionuclide 137-Cs. Behrens et al. predict a too late time of arrival but with lower activities that appear to more realistic. It important to note that these models carry the own simplifications and assumptions (e.g. see section 3.4 Caveats of the Behrens et al. (2012) study) and that recent measurements suggest that some of the Fukushima plume is being dispersed to the south rather than to the east in the Pacific (e.g. Kumamoto et al. (2014) open-access; more on this study in a forthcoming post).
Articles that confuse the conclusions of the Chinese study are a good example of poor reporting on an important subject. The example here was originally spawned by Energy News who have a history of inaccurate reporting on Fukushima and then propagated through the web by uncritical followers of the site.