Category Archives: Sample type

Most Recent Measurements of Plutonium in Pacific: Fukushima Fallout Undetectable

By Jay T. Cullen

@JayTCullen and @FukushimaInFORM

The purpose of this post is to report results from two recently published studies on plutonium releases from Fukushima to the Pacific Ocean. The post contributes to an ongoing series where results from peer-reviewed studies on the impact of the triple meltdowns at the Fukushima Dai-ichii nuclear power plant on the health of the Pacific ecosystem and residents of the west coast of North America are reported. A frequently asked question of those involved in monitoring the health of the North Pacific is why more measurements of the long lived, alpha-emitting isotopes of plutonium (239Pu half-life 24,100 years; 240Pu 6,570 years) are not being made given the potential for these isotopes to pose radiological health risks. Previous work indicates that 239+240Pu releases from Fukushima were about 100,000 and 5,000,000 times lower than releases from the Chernobyl disaster in 1986 and 20th century weapons testing respectively. Initial measurements of Pu isotopes in seawater and marine sediments off the coast from Fukushima indicated no detectable change occurred in Pu inventories in the western Pacific after the disaster. These two most recent studies monitored the activity and isotopic composition of Pu in seawater and marine sediments off of Japan from 2008-2013. Similar to earlier work these studies find that the release of Pu isotopes by the Fukushima accident to the Pacific Ocean has been negligible. The Fukushima signal is not detectable in the ocean off Japan relative to legacy sources from atmospheric weapons testing in the 20th century. Given these accumulating results 239+240Pu from Fukushima is unlikely to negatively impact the health of the Pacific Ocean ecosystem and levels in the environment from Fukushima will not pose a danger to the population of North America.
Continue reading Most Recent Measurements of Plutonium in Pacific: Fukushima Fallout Undetectable

Observing the Arrival of the Fukushima Contamination Plume in North American Coastal Waters

By Jay T. Cullen

@JayTCullen and @FukushimaInFORM

This short blog summarizes an open access paper published today reporting results from a Canadian monitoring program tasked with documenting the arrival of ocean borne Fukushima contamination along the North American Pacific coast. This diary is part of an ongoing effort to communicate the best science available on the impacts of the Fukushima Dai-ichi meltdowns on the environment. High quality measurements to look for Fukushima derived radiocesium were made in seawater in the North Pacific and Arctic Oceans from 2011 to early 2014. The authors concluded that:

  1. Fukushima derived radiocesium was first detected 1500 km west of British Columbia Canada in June 2012
  2. Contamination was detected on the continental shelf (near coastal waters) in June 2013
  3. By February 2014 Fukushima radiocesium was present at levels similar to preexisting weapons testing derived 137-Cs
  4. The timing of the arrival and levels of radiocesium in the contaminated plume are in reasonable agreement with existing ocean circulation model predictions
  5. These same models predict that total radiocesium levels from weapons testing fallout and Fukushima will likely reach maximum values of ~3-5 Becquerel per cubic meter (Bq m-3 of seawater in 2015-2016 and then decline to fallout background level of ~1 Bq m-3 by 2021
  6. Fukushima will increase northeastern Pacific water to levels last seen in the 1980’s but does not represent a threat to environmental or human health

Continue reading Observing the Arrival of the Fukushima Contamination Plume in North American Coastal Waters

Scientific Study of Radioactive Cesium Accumulation by Salmon

By Jay T. Cullen

@JayTCullen and @FukushimaInFORM

Male spawning phase Oncorhynchus nerka. When landlocked (freshwater phase) this sockeye salmon is referred to as kokanee.

 

The purpose of this post is to report a recently published study (behind pay wall) that examined how and how much radioactive cesium is accumulated by salmonids (e.g. salmon and trout). This post is part of an series started in 2013 to communicate the results of scientific research into the impact of the Fukushima Dai-ichi triple meltdowns on the environment. Yamamoto and colleagues carried out two experiments (one lake cage experiment and a laboratory experiment) to examine the accumulation of radiocesium from water and food by kokanee (Oncorhynchus nerka) and masu salmon (Oncorhynchus masou). The conclusions of the study were as follows:

Continue reading Scientific Study of Radioactive Cesium Accumulation by Salmon

Looking For Fukushima Contamination in Mushrooms and Soil of Western North America

By Jay T. Cullen

@JayTCullen

Chanterelle Cantharellus cibarius
 

The purpose of this diary is to report results from a recently published, peer reviewed study (behind paywall) examining the degree of Fukushima contamination in fungi and soil of western North America. The diary is the most recent contribution to an ongoing series which aims to provide evidence from scientific studies assessing the impact of the Fukushima Daiichi disaster on the environment and the health of residents of North America. Trappe and colleagues measured the activity of cesium isotopes (134-Cs half life ~ 2 years; 137-Cs half life ~30 years) in wild mushrooms, soil and leaf litter of the west coast from California up to Vancouver Island. The conclusions of the study were as follows:

  1. No activity measurements exceeded levels thought to impact human health
  2. 137-Cs activity increased in fungi and soil towards the north
  3. 134-Cs increased to the south in leaf litter
  4. Chanterelles did not significantly bioconcentrate Cs isotopes
  5. 137-Cs and 134-Cs activities were highly variable from sample to sample
  6. 137-Cs levels largely reflected non-Fukushima sources from either atmospheric weapons tests in the last century or the Chernobyl disaster in 1986

Continue reading Looking For Fukushima Contamination in Mushrooms and Soil of Western North America

Plutonium Inventories at Fukushima Dai-ichi Nuclear Power Plant and Mixed Oxide (MOX) Fuel at Unit 3

By Jay T. Cullen

The purpose of this post is to provide estimates of the plutonium (Pu) isotopes present at the Fukushima Dai-ichi nuclear power plant (NPP) at the beginning of the disaster in March 2011. The post is part of an ongoing effort to communicate facts about Fukushima obtained through scientific study of the impact of the meltdowns on the environment. Comments on this site and in other public forums highlight the fact that Unit 3 at the NPP was burning mixed oxide (MOX) fuel at the time of the accident which, because it is enriched in Pu, suggests that these releases are potentially more harmful. Here I report estimates of Pu present in the reactors (Units 1, 2 and 3) and spent fuel pools (Units 1-4) at the site based on burnup calculations. Because fission of low enriched uranium (LEU) fuel produces Pu isotopes during operation there was a significant amount of Pu on site in Units 1-4. During extended operation a MOX fuel burning reactor can produce multiple times the Pu of LEU but this was not so at the time of the Fukushima meltdowns. The amount of additional Pu present due to Unit 3’s MOX fuel is small compared to the other reactor cores and the inventory of the spent fuel pools. The differences between environmental impact of MOX versus LEU reactor core meltdown in this case are small. Estimates of the release of Pu isotopes from Fukushima, based on measurements of air, soil and water suggest 100,000 fold less was broadcast to the environment compared to Chernobyl and 5,000,000 fold lower than releases from nuclear weapons testing in the 20th century. Continue reading Plutonium Inventories at Fukushima Dai-ichi Nuclear Power Plant and Mixed Oxide (MOX) Fuel at Unit 3