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Seawater testing project ramps up
Citizen scientists aid in tracking coastal radiation
by Chris Bolster | reporter@prpeak.com

Published: Wednesday, October 8, 2014 12:42 PM PDT
A seawater testing project on BC’s coast is ramping up to record the arrival of Japanese radiation leaked into the sea from the Fukushima Daiichi nuclear power plant disaster.

On March 11, 2011, the plant on the north east coast of Japan was hit by a tsunami triggered by a 9.0 magnitude earthquake. Three of the six nuclear reactors at the plant went into meltdown and a day later started to leak radioactive material into the Pacific Ocean. It is known as the largest nuclear incident since Chernobyl in 1986.

Dr. Jay Cullen is a chemical oceanographer at the University of Victoria who is leading the three-year project.

Starting this month, Cullen and his team will be coordinating about 600 citizen scientist volunteers in 14 coastal communities who will be collecting seawater samples monthly to send to the lab.

“The project itself is building on the success of more modest testing programs the Department of Fisheries and Oceans (DFO) and Health Canada have been carrying out since the triple meltdown at Fukushima Daiichi in March 2011,” said Cullen.

DFO and Dr. John Smith have been making measurements in the north east Pacific and the Arctic oceans looking for radionuclides from Fukushima in seawater, he said.

Cesium-137, a signature isotope of Fukushima, was first detected about 1,500 kilometres offshore in 2012. In June 2013 it was detected off the west coast of Vancouver Island.

Cullen’s project will track the arrival of the plume of contaminated seawater being transported on North Pacific ocean currents.

“It’s to track its arrival and look for the maximum activities of these isotopes which will dictate what the risk is to the public,” Cullen said, adding that estimates suggest peak levels will reach BC during the next three years.

Scientist have measured low levels of radioactive material in seawater for decades.

“If you look at the activity of some of the isotopes which present the greatest health risks like Cesium-137 or Strontium-90 those levels peaked in the mid-1960s as a result of weapons testing,” said Cullen.

Currently there is only a slight trace of the chemicals from the disaster, he said.

“If you lived here in the 1970s or 80s the radioactivity of seawater and fish was likely greater than what we expect to be resulting from Fukushima,” he added.

Readers interested in the most recent scientific studies on the radiation-contaminated seawater or more information on the project, can visit Cullen’s blog or the study’s website.

Update on Fukushima Plutonium Releases to the Pacific Ocean

By Jay T. Cullen

This post reports on the most recent study of plutonium releases from Fukushima to the Pacific Ocean. The post contributes to an ongoing effort to report peer-reviewed studies on the impact of the triple meltdowns at the Fukushima Dai-ichii nuclear power plant on the health of the Pacific ecosystem and residents of the west coast of North America. Plutonium is an alpha-emitting isotope that carries significant radiological health risks if internalized with risk of exposure increasing with the activity of Pu isotopes in the environment. Previous work indicates that 239,240-Pu releases from Fukushima were about 100,000 and 5,000,000 times lower than releases from the Chernobyl disaster in 1986 and 20th century weapons testing respectively. Initial measurements of Pu isotopes in seawater and marine sediments off the coast from Fukushima indicated no detectable change occurred in Pu inventories in the western Pacific after the disaster. More recent and more expansive work supports earlier studies drawing the conclusion that up to two years after the accident the release of Pu isotopes by the Fukushima accident to the Pacific Ocean has been negligible.


A paper by Bu and colleagues was recently published in the peer-reviewed journal Environmental Science and Technology which investigated the activity of Pu isotopes marine sediments collected within 30 km of the Fukushima reactor sites. 239,240,241-Pu and radiocesium isotopes (134-Cs and 137-Cs) were measured. Given that Pu is a particle reactive element that would tend to be concentrated in sediments such measurements should help to determine the extent and degree of Fukushima derived Pu in the marine environment. Sample collection sites are indicated in the map below.

Map showing the locations for (a) sediment samples collected within the 30 km zone around the FDNPP site and (b) sediment samples collected outside the 30 km zone around the FDNPP site in previously published studies by Bu and colleagues.
Relatively high activities of 134-Cs and 137-Cs and a decay corrected ratio near 1 indicated that the sediments were indeed contaminated with Fukushima derived radionuclides.
137-Cs activities and 134-Cs/137-Cs activity ratios in the marine sediments (decay corrected to 15 March 2011) determined by Bu et al. 2014. The blue dashed line represents the 134Cs/137Cs activity ratio fingerprint of the radiocesium released by the Fukushima disaster.
In contrast to the clear imprint of Fukushima derived Cs on the marine sediments the activities of 239,240-Pu and 241-Pu were low compared with the background level before the accident. The Pu activity ratios (240-Pu/239-Pu and 241-Pu/239-Pu) suggested that the Pu detected was the result of global fallout and the pacific proving ground (PPG) close-in fallout resulting from atmospheric weapons testing in the 20th century. The following figure is a mixing diagram that helps to determine the relative contributions to the observed Pu contamination of marine sediments off the Japanese coast.
Mixing plot of 241-Pu/239-Pu atom ratio vs 240-Pu/239-Pu activity ratio in Fukushima sediments compared with Pu compositions of global weapons fallout, Fukushima release, and the Pacific Proving Ground weapons fallout. The closed orange circles (soil and litter samples) and closed black circles (aerosol samples) represent the Fukushima source; the closed pink circle represents the global weapons test fallout; the closed blue circles represent the surface sediment samples collected outside the 30 km zone; the open black circles represent sediment samples within 30 km of the Fukushima site; the closed violet circle represents Sagami Bay sediment samples; the closed wine colored circles represent Pacific Proving Ground source.
The mixing diagram indicates that the isotopic ratio of Pu in marine sediments is inconsistent with a significant release of Fukushima Pu to the marine environment. The isotopic composition of Pu in marine sediments is consistent with Pu deposited during atmospheric weapons testing in the last century.

While initial releases from the plant and ongoing releases due to groundwater infiltration and terrestrial runoff have been negligible thus far according the authors they rightly point out that significant inventories of Pu are insecurely stored at the Fukushima site. So far estimates suggest that about 2.3×10^9 Bq of 239,240-Pu or 580 milligrams of the isotopes have been broadcast to the environment from Fukushima. Bu et al. (2014) estimate that contained within the roughly 270,000 tons of radioactive liquid waste stored in large tanks at Fukushima there exists approximately a further 1×10^8 Bq of 239,240-Pu. Given that future earthquakes or other events could mobilize this Pu, continued monitoring of Pu isotopes in the marine environment is necessary and prudent.

Authors Lower Fukushima Cesium in North Pacific By Order of Magnitude

By Jay T. Cullen

Introduction

One of the goals of the InFORM project is to make measurements of radionuclides in the North Pacific Ocean to determine maximum activities that will determine impacts on the marine ecosystem and residents of the west coast. The purpose of this post is to bring to the attention of readers a recently published correction to a prominent model that predicts the activity of Fukushima derived Cesium-137 (137-Cs, half life ~30 years) in seawater of the North Pacific. The diary is part of an ongoing series aimed at discussing research addressing the impact of the Fukushima nuclear disaster on the health of the North Pacific Ocean and inhabitants of North America’s west coast. Predictions of a model by Rossi and colleagues published in Deep-Sea Research in 2013 of the evolution of the plume of seawater contaminated by the Fukushima triple meltdowns are an order of magnitude too high. Rather than a range of ~1-30 Bq/m^3 reported previously maximum activities off the west coast of North America are likely to be ~3 Bq/m^3 or about more than 25 times lower than maximum activities measured in the Pacific in the mid-20th century resulting from atmospheric weapons tests. These activities are not likely to represent significant radiological health risks to the North Pacific ecosystem or residents of the North American west coast.


A paper by Rossi et al. (2013) used a Lagrangian model to predict the temporal and spatial evolution of the seawater plume contaminated by the Fukushima nuclear disaster beginning in March 2011. The model predicted a range of 10-30 Bq/m^3 137-Cs in waters off the coast of North America at 49 degrees North latitude as demonstrated in the figure shown below:

Activities of 137-Cs predicted by the Rossi et al. (2013) model on the continental shelves of North America at two latitudes and off Hawaii over time.

This model predicted higher maximum 137-Cs activities in seawater in the North Pacific compared with a similar model published by Behrens et al. (2012) that had maximum activities off of North America reaching only ~1-2 Bq/m^3.

Recently, after comments from Professor Michio Aoyama of Japan, Rossi and colleagues recognized an error in their model and have published a correction to their 2013 study here. The error resulted in a factor of 10 overestimation of maximum activities of 137-Cs in the Pacific such that maximum 137-Cs off N. America will likely be between 1 and 3 Bq/m^3. The corrections to the model do not affect the conclusions of the study and results from the 2013 study are easy scaled to the more accurate values given the Langrangian approach used by the authors in the original work.

The figure below shows the time evolution of the plume at various latitudes along the international date line and compares the model output with measurements made by Aoyama et al. (2013) along the international dateline at about 40 degrees N in 2012.

Activities of 137-Cs predicted by the Rossi et al. model along the international dateline in the N. Pacific over time at various latitudes.

The factor of 10 lower activity correction better agrees with the Behrens et al. (2012) modeling study and measurements of 137-Cs in seawater made by Japanese and North American scientists.

Maximum activities of ~1-3 Bq/m^3 as the heart of the contaminated plume reaches the North American coast in the coming 2 year period are roughly 25-fold lower than 137-Cs activities in the North Pacific circa 1960 resulting from atmospheric weapons testing. Therefore, it is unlikely that 137-Cs activities of 3 Bq/m^3 or associated radionuclides released at lower total activities from Fukushima will represent significant health risks to the North Pacific ecosystem.

Ongoing monitoring of radionuclide activities in the North Pacific is required to ground-truth models of Pacific Ocean circulation and plume evolution and to provide the best information to determine likely impact to residents of North America.

Fukushima Radionuclides in Pacific Albacore Tuna Off the US Coast

Tuna and gamma spectra. (Neville et al. 2014)
Tuna and gamma spectra. (Neville et al. 2014)

By Jay T. Cullen

Introduction

As part of an ongoing series documenting the impacts of the Fukushima disaster on the North Pacific and west coast, this post summarizes a recently published study by Delvan Neville and colleagues in the peer-reviewed journal Environmental Science and Technology. The paper reports measurements of Cesium-134 and Cesium-137 in 26 albacore tuna caught off the west coast of North America between 2008 and summer 2012. Because of its relatively short half-life (~2 years) 134-Cs is an unambiguous tracer of radionuclides released from the Fukushima Dai-ichi disaster which began in March 2011. Fish collected in 2011 and 2012 had higher 134-Cs and 137-Cs that was due to Fukushima sourced cesium in the Pacific. Fish collected in 2008-2009 had lower 137-Cs activities that largely reflected historic releases of the isotope from atmospheric nuclear weapons testing in the 20th century. The authors conclude that given the highest levels of Cs isotopes measured in albacore tuna, human consumption of the fish would not not represent a significant increase in annual radiation dose. The corresponding radiological health risk due to Fukushima derived radiocesium in these tuna is, therefore, very small. Continue reading Fukushima Radionuclides in Pacific Albacore Tuna Off the US Coast

More Measurements of Southward Transport of the Fukushima Contaminant Plume in the Western Pacific

by Jay T. Cullen

This post is part of an ongoing series that endeavors to report measurements of Fukushima derived radionuclides in the environment to help determine the likely impact on ecosystem and public health in western North America. One of the goals of the InFORM project is to provide quality measurements of Fukushima derived radionuclides in the North Pacific to help verify model predictions of ecosystem and public health impacts of the disaster. The purpose of this post is to summarize results of a recent peer reviewed study by Kaeriyama and colleagues published in Environmental Science & Technology who measured radioactive isotopes of cesium (137-Cs half life ~30 yr and 134-Cs half life ~ 2 yr) in the western North Pacific Ocean to help track the location and movement of the Fukushima contaminated seawater plume.

Continue reading More Measurements of Southward Transport of the Fukushima Contaminant Plume in the Western Pacific